π Complexes of Transition Metals by Priv.-Doz. Dr. Günter Häfelinger (auth.)

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By Priv.-Doz. Dr. Günter Häfelinger (auth.)

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A. : Chem. Rev. 69, 157 (1969). 10) Coulson, C. : Nature 221, 1106 (1969). , Raimondi, D. , Reinhardt, W. : IBM Res. Rept. RJ - 431 (1962). 12) Quin, L. , Bryson, J. , Moreland, C. : J. Am. Chem. Soc. 91, 3308 (1969). la) Brown, D. : J. Chem. Soc. : Angew. Chem. 78, 907 (1966). IS) Bart, J. C. , Daly, J. : Angew. Chem. 80, 843 (1968). : Angew. Chem. 75, 669 (1963). 17) Daly, J. : Chem. Commun. 1969, 1057. : Angew. Chem. 81, 783 (1969). 19) _ Bugg, C. : Angew. Chem. 82, 933 (1970). : Z. Naturforsch.

Susuki and Tsuji reported that addition of carbon tetrachloride to olefins and carbonylation are catalyzed by dinuclear metal carbonyl complexes like [Tr-CsHsFe(CO)2]2 and [Tr-CsHsMo(CO)3]2 ss,s9). COC1 R-CH=CH2 + CO + CC14 J R-C-CH2CC13 I H 54 Organic Synthesis by Means of Transition Metal Complexes In these reactions, the splitting of the metal-metal bond with carbon tetrachloride is assumed. The homolysis of the covalent carbon-chlorine bond is closely related to the formation of free radicals.

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